Eccentric metallo-dielectric core-shell nanoparticles for light guiding and switching
High Refractive Index Dielectric (HRID) nanoparticles (NPs) have been proposed as an alternative to metallic ones due to their low absorption and magnetodielectric response in the VIS and NIR ranges. Important scattering directionality (SD) effects can be obtained and systems constituted by dimers of HRID NPs present switching effects by playing with the polarization, frequency or intensity of the incident radiation.
In this work, we show that SD effects can be achieved with a single eccentric metallo-HRID core-shell nanoparticle, in particular a Ag-Si core-shell nanoparticle, when its metallic core is shifted from its center. Depending on this shift, these scattering units show different directionality behaviors: 1) If the core’s shift is parallel to the propagation direction of the incident radiation, SD conditions can be enhanced. 2) If it is perpendicular to the direction of the incoming beam, those scattering units can operate as switching devices. In fact, we report a rotation of the main scattering lobe either clockwise or counterclockwise depending on the polarization of the incident radiation. This suggests that this sort of eccentric core-shell NPs show efficient configurations for redirecting the incident radiation to certain directions respect to that of forward and backward. This behavior can be exploited for building operational switching devices, whose “on”/”off” states only depend on the polarization of the incoming wave. The analysis of the scattered radiation has been performed at 90º with respect to the incident radiation. This configuration avoids any parasitic effect due to the incident beam. Figure 1 shows the scattering diagrams for an isolated eccentric metallo-dielectric core-shell nanoparticle of radius Rext = 230 nm, whose core (Rcore = 70nm) has been shifted along the X-axis (perpendicular to the incident wave direction. See the rest of details in the figure caption). By swapping the polarization of the incident radiation from s (perpendicular to the scattering plane, ZX) to p (parallel to the scattering plane) and fixing a minimum intensity threshold (which will be considered as the “off” state of the device), the intensity of the scattered radiation at 90° goes from a “high” (“on” state) to a “low” (“off” state) level.
We also obtain both cumulative radiation guiding effects, by using chains of these scattering units, and, in the case of 1D periodic arrays, redirection of diffracted intensity as a consequence of “induced” blazing effects. Figure 2 (a) and (b) show near and far field performances of a chain of 6 of the proposed scattering units. This evidences the enormous potential of the directionality properties of these nanostructures, paving the way for new nanoantenna designs. Figure 2 (c) shows the scattering patterns of a system built with 5 core-shell NPs, either concentric or eccentric, distributed as a 1D array (see figure caption for details). A redirection of the diffracted intensity, due to the “induced” geometrical anisotropy of the isolated NP, can be observed.
The scattering units proposed in this research, constitute possible new building-blocks for more complex systems for applications in optical communications, solar energy harvesting and light guiding at the nanoscale level.
Ángela I. Barreda1, Yael Gutiérrez1, Juan M. Sanz1,2, Francisco González1, Fernando Moreno1
1Grupo de Óptica, Departamento de Física Aplicada, Universidad de Cantabria,
Facultad de Ciencias, Avda. Los Castros s/n, 39005, Santander, Spain
2Departamento de I+D, Textil Santanderina,
S.A., Avenida Textil Santanderina, s/n, 39500, Cabezón de la Sal, Spain
Light guiding and switching using eccentric core-shell geometries.
Barreda ÁI, Gutiérrez Y, Sanz JM, González F, Moreno F
Sci Rep. 2017 Sep 11
|How to design a plasmonic sensor more sensitive to… Noble metal nanoparticles (NPs) such as Au NPs and Ag NPs support localized surface plasmon resonances (LSPRs), which are the light-coupled coherent oscillations of free electrons confined within the NPs.…|
|Compact, all-optical, Terahertz wave generator Terahertz (THz) wave is a kind of invisible light that has the frequency of about 1012 Hz. THz wave can path through different materials with small absorption or reflection, therefore…|
|What happens when quick-response code meets with… Today, diabetes mellitus and hypoglycemia severely harm human health and daily life. For example, the diabetes increases the risk of cardiovascular disease and of early death. However, conventional glucose sensors…|
|Harnessing Förster energy transfer Our fascination with light, matter and their mutual interactions has been the driving force behind the advent of new optical materials, ranging from a variety of organic and inorganic dielectrics…|
|SERS substrates by vacuum-free dealloying of… Plasmonics has become an important photonic device due to the advancement of fabrication technologies in recent decades. It has many applications including solar cells, nonlinear optics, metamaterials, photocatalysts, and surface-enhanced…|
|A photothermal optical sensor enables measurement of… Examining blood sample is like looking over the index of a book on the health of humans. For example, measuring cholesterol concentration in blood enables detection of hyperlipidemia, which is…|